High-Efficiency Second-Harmonic Generation from Hybrid Light-Matter States

Chervy, Thibault; Xu, Jialiang; Duan, Yulong; Wang, Chunliang; Mager, Loic; Frerejean, Maurice; Münninghoff, Joris A. W.; Tinnemans, Paul; Hutchison, James Andell; Genet, Cyriaque; Rowan, Alan E.; Rasing, Theo; Ebbesen, Thomas

doi:10.1021/acs.nanolett.6b02567

High-Efficiency Second-Harmonic Generation from Hybrid Light-Matter States

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CHERVY, Thibault, XU, Jialiang, DUAN, Yulong, WANG, Chunliang, MAGER, Loic, FREREJEAN, Maurice, MÜNNINGHOFF, Joris A. W., TINNEMANS, Paul, HUTCHISON, James Andell, GENET, Cyriaque, ROWAN, Alan E., RASING, Theo et EBBESEN, Thomas, 2016. High-Efficiency Second-Harmonic Generation from Hybrid Light-Matter States. Nano Letters [en ligne]. 21 novembre 2016. Vol. 16, n° 12pp. 7352-7356. [Consultésans date]. DOI 10.1021/acs.nanolett.6b02567. Consulté de : https://pubs.acs.org/doi/abs/10.1021/acs.nanolett.6b025671. .

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Auteurs	Thibault Chervy Jialiang Xu Yulong Duan Chunliang Wang Loic Mager Maurice Frerejean Joris A. W. Münninghoff Paul Tinnemans James Andell Hutchison Cyriaque Genet Alan E. Rowan Theo Rasing Thomas Ebbesen
Unité de recherche du site	Institut de Science et d'Ingénierie Supramoléculaires - ISIS - UMR7006 Institut de Physique et Chimie des Matériaux de Strasbourg - IPCMS - UMR7504
Langue	en
Volume	16
Numéro	12
Page de début	7352
Page de fin	7356
Date de première publication	2016-11-11
Date de parution	2016-11-21
ISSN	1530-6984 1530-6992
Titre de la source (revue, livre…)	Nano Letters
Résumé	We report a novel approach to modify the second order nonlinear optical (NLO) susceptibility of organic nanofiber crystals by hybridization with the optical modes of microcavities in the strong coupling regime. The wavelength dependence of the SHG Show moreWe report a novel approach to modify the second order nonlinear optical (NLO) susceptibility of organic nanofiber crystals by hybridization with the optical modes of microcavities in the strong coupling regime. The wavelength dependence of the SHG efficiency displays two intense peaks corresponding to the so-formed light-matter hybrid states. Our results demonstrate an enhancement of the resonant SHG efficiency of the lower polariton by 2 orders of magnitude for the collectively coupled molecules as compared to that of the same material outside the microcavity. This study is a proof of principle that opens a new direction for NLO of organic materials in subwavelength resonators. Show less
DOI	10.1021/acs.nanolett.6b02567
Éditeur	American Chemical Society
URL éditeur	https://pubs.acs.org/doi/abs/10.1021/acs.nanolett.6b02567
Titre abrégé de la source	Nano Lett.
Type de publication	ACL
Projet(s) de recherche ANR	ANR-10-IDEX-0002-02 ANR-10-EQPX-52-01 ANR-11-LABX-0058_NIE
Projet(s) de recherche européen(s)	EC/FP7/227577///PLASMONICS
Topic	Aucun
Unité de recherche extérieure au site	School of Chemical Engineering and Technology, Tianjin University, Yaguan Road 135, 300350 Tianjin, People’s Republic of China Institute for Molecules and Materials (IMM), Radboud University, Heyendaalseweg 135, 6525AJ Nijmegen, The Netherlands Institute for Molecules and Materials (IMM), Radboud University, Heyendaalsewe
Équipes de recherche	E1 - DON : Département d'optique ultra-rapide et de nanophotonique
Fonction	aut -clb
Identifiant idREF	224351702 150567634 075088843 086037536
Audience	Non spécifiée
URL	https://univoak.eu/islandora/object/islandora:72151